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There's a lot of good documentaries on there between originals like Imagineering Story, Prop Culture, the Howard Ashman biography and that show looking behind the scenes at Animal Kingdom and older stuff like Waking Sleeping Beauty and the Sherman Brothers documentary.
Also if you want some weird shit beyond the typical "Troy McClure-tier live-action comedies", that Mouseketeers at Disney World thing is just this bizarre time capsule of the 1970s that includes the original commercials as if they just randomly digitized some tape they found in somebody's closet.