>Spiderman
2 (GC/PS2/Xbox version), Web of Shadows, PS4. I liked some others, but off the top of my head these are the best ones. I do have nostalgia for the first movie's game though.
>X-Men
The Origins:Wolverine tie-in is actuslly not bad. I love the sequence where you fight a Sentinel. To all you zoomers: movie tie-in games usually injected a lot of stuff that wasn't in the actual movie, otherwise you'd have 3-4 levels of action. Also, they were being made while the movie was made, therefore the devs wouldn't necessarily have all the plot details aside from the obvious (I.e. Green Goblin kidnaps MJ). So yes, the Origins game has Sentinels! It gets very repetitive, but it's mainly just fun to see M-rated Wolverine carnage. 6/10 game IMO.
>Batman
Arkham series of course, you can skip Origins.